In order for you to create synced charts, you need to use the same type of axis in each chart and each chart needs to have the same horizontal data, so that the axes end up with the same categories set.
For example you cannot provide 2010, 2011 and 2012 for the first chart and 2011, 2012 and 2013 for the second chart, because the axes will end up with different categories and no alignment of data will be achieved. You need to supply both charts with 2010, 2011, 2012, 2013.
After syncing the horizontal axis categories, almost full alignment will be achieved automatically. Small displacements may occur of you have the vertical axes visible and they have different ranges. In the image you attached, the axes are collapsed so this is not expected to happen.
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